• Title of article

    Aromatic Ring-Opening of 2-Fluorobenzothiophenes by Alkyllithiums

  • Author/Authors

    Belley، Michel نويسنده , , Douida، Zohra نويسنده , , Mancuso، John نويسنده , , Vleeschauwer، Marc De نويسنده ,

  • Issue Information
    روزنامه با شماره پیاپی سال 2005
  • Pages
    -246
  • From page
    247
  • To page
    0
  • Abstract
    Diphenylacetylenes are obtained when alkyllithium ­reagents are added to 3-aryl-2-fluorobenzothiophenes at low temperature. The aromatic ring-opening mechanism involves a nucleophilic addition of the alkyllithium to the sulfur atom of the thiophene. The resulting 2,2-diaryl-1-fluorovinyl anion subsequently undergoes a Fritsch-Buttenburg-Wiechell rearrangement to ­afford the diphenylacetylene.
  • Keywords
    alkyllithium reagents , addition to sulfur , benzothiophenes , ring-opening , Fritsch-Buttenberg-Wiechell rearrangements
  • Journal title
    Synlett
  • Serial Year
    2005
  • Journal title
    Synlett
  • Record number

    110420