Author/Authors :
Zhixin Guo، نويسنده , , Yuliang Li، نويسنده , , Fenglian Bai، نويسنده , , Jimin Yan a، نويسنده , , Zhongxin Ge، نويسنده , , Daoben Zhu، نويسنده , , Jinhai Si، نويسنده , , Peixian Ye، نويسنده , , Lingxuan Wang، نويسنده , , Tiankai Li، نويسنده ,
Abstract :
The Langmuir and Langmuir–Blodgett (LB) films of a novel crowned [60]fullero-pyrrolidine(CFP) were produced in different conditions. Macroscopic second-harmonic generation of the LB film was investigated by means of AM1 Hamiltonian as well as experiments. The monolayer LB film displayed a periodic fringe pattern. A linear dependence of second-harmonic intensity on the number of layers was observed. The second-order molecular susceptibility χ(2) and hyperpolarizability β were evaluated to be 3.2×10−8 and