Title of article :
Theory of the relation between inelastic scanning tunneling spectroscopy of adsorbates and their vibrational deexcitation
Author/Authors :
Mingo، نويسنده , , N and Makoshi، نويسنده , , K and Mii، نويسنده , , T and Ueba، نويسنده , , H، نويسنده ,
Issue Information :
هفته نامه با شماره پیاپی سال 2001
Abstract :
We show how the rate for controlled excitation of adsorbate vibrational modes by scanning tunneling microscope can be quantitatively related to the lifetimes of these modes when deexciting by electron–hole pair mechanism. To this end we present a Green function formalism that accounts for the two processes in a unified way. A model calculation for an adsorbate like CO is studied and compared with existing experimental results.
Keywords :
CARBON MONOXIDE , Surface electronic phenomena (work function , Surface potential , etc.) , Surface states , Green’s function methods , Tunneling , Vibrations of adsorbed molecules , Metallic surfaces
Journal title :
Surface Science
Journal title :
Surface Science