Title of article
Effects of electron levels broadening and electron temperature in tunnel structures based on metal nanoclusters
Author/Authors
Babich، نويسنده , , A.V. and Pogosov، نويسنده , , V.V.، نويسنده ,
Issue Information
هفته نامه با شماره پیاپی سال 2010
Pages
7
From page
210
To page
216
Abstract
We study the influence of energy levels broadening and electron subsystem overheating in island electrode (cluster) on current–voltage characteristics of three-electrode structure. A calculation scheme for broadening effect in one-dimensional case is suggested. Estimation of broadening is performed for electron levels in disc-like and spherical gold clusters. Within the two-temperature model of metallic cluster and by using a size dependence of the Debye frequency the effective electron temperature as a function of bias voltage is found approximately. For helium temperature of ion subsystem, the heating temperature of electrons in a quantum disc is almost one order of magnitude higher than that in a sphere; it achieves thousands of Kelvin. We suggest that the effects of broadening and electron overheating are responsible for the smoothing of current–voltage curves, which is observed experimentally at low temperatures in structures based on clusters consisting of accountable number of atoms. However, a role of the broadening is much more significant.
Keywords
electron density , Equilibrium thermodynamics and statistical mechanics , Semi-empirical models and model calculations , Excitation spectra calculations , Tunneling
Journal title
Surface Science
Serial Year
2010
Journal title
Surface Science
Record number
1705370
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