Title of article
Methane reforming to syngas over LaNixFe1−xO3 (0 ≤ x ≤ 1) mixed-oxide perovskites in the presence of CO2 and O2
Author/Authors
Hamidreza Arandiyan، نويسنده , , Hamidreza and Li، نويسنده , , Junhua and Ma، نويسنده , , Lei and Hashemnejad، نويسنده , , S.M. and Mirzaei، نويسنده , , M.Z. and Chen، نويسنده , , Jinghuan and Chang، نويسنده , , Huazhen and Liu، نويسنده , , Caixia and Wang، نويسنده , , Chizhong and Chen، نويسنده , , Liang، نويسنده ,
Issue Information
روزنامه با شماره پیاپی سال 2012
Pages
12
From page
2103
To page
2114
Abstract
The perovskite metal-oxides LaNixFe1−xO3 (0 ≤ x ≤1) were synthesized by a sol–gel method and investigated for the DR, POM, and CRM into synthesis gas. The catalysts were characterized by using XRD, BET, CA, SEM, EDS, HR-TEM, EDX and TPR in order to investigate the influence of the preparation parameters and evaluation condition. LaNi0.4Fe0.6O3 showed great stability, and fewer carbon deposits were detected on the spent catalyst after 1800 min evaluation on TOS. The effect of GHSV on the catalytic performance was investigated. The results obtained showed the H2/CO molar-ratio was around 0.9, 1.7, and 1.1 over different catalysts for DR, POM and CRM, respectively.
Keywords
Perovskite catalyst , Dry reforming , Syngas , Combined reforming , partial oxidation
Journal title
Journal of Industrial and Engineering Chemistry
Serial Year
2012
Journal title
Journal of Industrial and Engineering Chemistry
Record number
1710507
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