Title of article :
Intramolecular energy flow in the condensed phase: effects of dephasing on localization in the quantum stochastic pump model
Author/Authors :
Leitner، نويسنده , , David M. and Wolynes، نويسنده , , Peter G.، نويسنده ,
Issue Information :
روزنامه با شماره پیاپی سال 1997
Abstract :
Stochastic pump models have been widely used to describe the classical dynamics of isolated, multidimensional weakly chaotic systems, such as the nuclear motion of a molecule in a regime of weak rovibrational coupling. We recently showed that quantization severely restricts energy flow in the stochastic pump model. We show here how introducing a weak external noise mimicking the effect of dephasing collisions to the quantum stochastic pump model has dramatic consequences for the flow.
Journal title :
Chemical Physics Letters
Journal title :
Chemical Physics Letters