• Title of article

    Tensor propagator with weight-selected paths for quantum dissipative dynamics with long-memory kernels

  • Author/Authors

    Sim، نويسنده , , Eunji and Makri، نويسنده , , Nancy، نويسنده ,

  • Issue Information
    روزنامه با شماره پیاپی سال 1996
  • Pages
    7
  • From page
    224
  • To page
    230
  • Abstract
    The tensor multiplication scheme, which allows iterative evaluation of the path integral for quantum dissipative dynamics, is extended to processes involving long-memory kernels such as those occurring in low-frequency solvents. Rather than propagating the augmented reduced density tensor in full-dimensional space, we propose here including in the propagator tensor only those path segments which enter the path integral with appreciable weight. The appropriate path segments are selected according to their weights by importance sampling. Elimination of the vast majority of paths which make negligible contribution in the path integral results in dramatic reduction of the required storage.
  • Journal title
    Chemical Physics Letters
  • Serial Year
    1996
  • Journal title
    Chemical Physics Letters
  • Record number

    1775901