Title of article
Two-dimensional line-shape analysis of photon-echo signal
Author/Authors
Okumura، نويسنده , , Ko and Tokmakoff، نويسنده , , Andrei and Tanimura، نويسنده , , Yoshitaka، نويسنده ,
Issue Information
روزنامه با شماره پیاپی سال 1999
Pages
8
From page
488
To page
495
Abstract
We analyze the two-dimensional (2D) line shape obtained by 2D Fourier transforming the time-domain response of a photon-echo signal as a function of the two coherence periods, t1 and t3. The line shape obtained for a two-level system with homogeneous and inhomogeneous broadening is shown to be sensitive to the magnitude of both of these line-broadening mechanisms. It is shown that the ellipticity of the 2D line shape can be related to the ratio of homogeneous to inhomogeneous broadening.
Journal title
Chemical Physics Letters
Serial Year
1999
Journal title
Chemical Physics Letters
Record number
1780357
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