• Title of article

    Detection of unusual ΔHOMO < ΔLUMO relationship in tetrapyrrolic cis- and trans-doubly N-confused porphyrins

  • Author/Authors

    Muranaka، نويسنده , , Atsuya and Homma، نويسنده , , Shigetsugu and Maeda، نويسنده , , Hiromitsu and Furuta، نويسنده , , Hiroyuki and Kobayashi، نويسنده , , Nagao، نويسنده ,

  • Issue Information
    روزنامه با شماره پیاپی سال 2008
  • Pages
    4
  • From page
    495
  • To page
    498
  • Abstract
    A plus-to-minus MCD sign in ascending energy has been detected for the Q bands of the copper(III) complexes of doubly N-confused porphyrin (cis- and trans-1). An unusual ΔHOMO < ΔLUMO relationship for tetrapyrrolic porphyrins was calculated using the HF, DFT, and semi-empirical methods. By applying the Michl’s perimeter model, the observed MCD pattern was successfully explained by the computational results.
  • Journal title
    Chemical Physics Letters
  • Serial Year
    2008
  • Journal title
    Chemical Physics Letters
  • Record number

    1924594