• Title of article

    Enhanced quantum entanglement in the non-Markovian dynamics of biomolecular excitons

  • Author/Authors

    Thorwart، نويسنده , , M. and Eckel، نويسنده , , J. and Reina، نويسنده , , J.H. and Nalbach، نويسنده , , P. and Weiss، نويسنده , , S.، نويسنده ,

  • Issue Information
    روزنامه با شماره پیاپی سال 2009
  • Pages
    4
  • From page
    234
  • To page
    237
  • Abstract
    We show that quantum coherence of biomolecular excitons is maintained over exceedingly long times due to the constructive role of their non-Markovian protein-solvent environment. Using a numerically exact approach, we demonstrate that a slow quantum bath helps to sustain quantum entanglement of two pairs of Fِrster coupled excitons, in contrast to a Markovian environment. We consider the cross-over from a fast to a slow bath and from weak to strong dissipation and show that a slow bath can generate robust entanglement. This persists to surprisingly high temperatures, even higher than the excitonic gap and is absent for a Markovian bath.
  • Journal title
    Chemical Physics Letters
  • Serial Year
    2009
  • Journal title
    Chemical Physics Letters
  • Record number

    1927315