Title of article :
Molecular photoelectron angular distributions with intense attosecond circularly polarized UV laser pulses
Author/Authors :
Yuan، نويسنده , , Kai-Jun and Chelkowski، نويسنده , , Szczepan and Bandrauk، نويسنده , , André D.، نويسنده ,
Issue Information :
روزنامه با شماره پیاپی سال 2014
Abstract :
We investigate effects of intermediate resonant electronic states on molecular photoelectron angular distributions (MPADs) by intense circularly polarized attosecond UV laser pulses. Simulations are performed on aligned H 2 + by numerically solving the corresponding three dimensional time dependent Schrِdinger equations. MPADs exhibit signature of rotations, which is shown to be critically sensitive to the symmetry of the intermediate resonant electronic state and the pulse intensity. This sensitivity is attributed to the coherent population transfer in the initial and intermediate resonant states, thus suggesting a method to control molecular photoionization on attosecond time scale.
Journal title :
Chemical Physics Letters
Journal title :
Chemical Physics Letters