Title of article :
Frequency dependent shear compliance of TaS3: Depinning relaxation spectra and search for a glass transition
Author/Authors :
Zhan، نويسنده , , X. and Brill، نويسنده , , J.W.، نويسنده ,
Issue Information :
دوماهنامه با شماره پیاپی سال 1999
Pages :
4
From page :
2671
To page :
2674
Abstract :
At T ≈ 100 K, the magnitude of the shear compliance of TaS3 increases by 25% with charge-density-wave (CDW) depinning by a dc voltage. We have measured the strain frequency dependence of the complex compliance (j) at different voltages, and fit it to distributions of Debye relaxation modes. The sensitivity of the compliance to the structure of the CDW suggests that it would also be sensitive to a glass transition. However, we find that both the real and imaginary parts of j are independent of frequency (within 1%) when the CDW remains pinned for 8 K < T < 70 K. j is also independent (0.1 %) of the frequency of small applied voltages, for which the dielectric constant varies greatly. Therefore, if there is a glass transition at these temperatures, these results imply that either it does not involve rearrangement of the CDW domain structure or that the elastic response time remains > l s for the pinned CDW.
Keywords :
Acoustic measurements , Transition metal chalcogenides , Glass transitions , charge density waves
Journal title :
Synthetic Metals
Serial Year :
1999
Journal title :
Synthetic Metals
Record number :
2073269
Link To Document :
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