Output power enhancement of Rhodamine 6G dye laser by colloidal gold nanoparticles

Abstract. Improvement of the eciency of a Rhodamine 6G dye laser by adding proper concentrations of gold colloidal nanoparticles into the dye solution has experimentally been investigated. Gold colloidal nanoparticles, due to their strong plasmonic peak in the visible region, are expected to have a considerable interaction with Rhodamine 6G dye molecules with broad emission spectrum in the visible range. It is shown that with addition of enough low concentrations (less than 0.4 M/l) of gold nanoparticles to the dye solution, both the output power and the eciency of the dye laser increase. The best improvement of the laser eciency reaches 15%. Two amplifying mechanisms exist for eciency improvement by the nanoparticles, which are resonant energy transfer from the plasmonic nanoparticles to the dye molecules and the high near eld around the nanoparticles. The results indicate that in low concentrations of gold nanoparticles, the amplifying mechanisms dominate the dissipating mechanism of scattering of the pumped light by the nanoparticles. This leads to the eciency improvement by addition of the nanoparticles.