PLUTON: A Three-Group Model for the Radial Distribution of Plutonium, Burnup, and Power Profiles in Highly Irradiated LWR Fuel Rods

A three-group model (PLUTON) is described, which predicts the power density distribution, plutonium buildup, and burnup profiles across the fuel pellet radius as a function of in-pile time and parameters characterizing the type of reactor system with respect to fuel temperature and changes of density during the irradiation period. The PLUTON model is a part of two fuel performance codes (ASFAD and FEMAXIV), which provide all necessary input for this model, mainly local temperatures and fuel matrix density across the radius. Comparisons between measurements and predictions of the PLUTON model are made on fuels with enrichments in the range 2.9 to 8.25% and with burnup between 21 000 and 64 000 MWd/t. It is shown that the PLUTON predictions are in good agreement with measurements as well as with predictions of the well-known TUBRNP model. The proposed model is flexibly applicable for all types of light water reactor (LWR) fuels, including mixed oxide, and for fuel tested in the Organization for Economic Corporation and Developmentʹs Halden heavy water reactor. The PLUTON three-group model is based on analytical (theoretical) consideration of neutron absorption in a resonant region of the fuel in its apparent form. It makes the model more flexible in comparison with the semi-empirical TUBRNP one-group model and allows the physically based model analysis of commercial LWR-type fuels at high burnup as well as analysis of experimental fuel rods tested in the Halden heavy water reactor, which is one of the main test reactors in the world. The differences in fuel behavior in the Halden reactor in terms of burnup distribution and plutonium buildup can be more clearly understood with the PLUTON model.