This paper reports on preparation of a magnetically anisotropic polycrystalline hexaferrite, Sr

Ca

Fe

O

, whose orientation degree is as high as 100%. The preparation uses standard ceramic techniques, including wet pressing and flowing-oxygen sintering. In this process, Ca

ions are substituted for Sr

ions in SrFe

O

by adding minimum impurities (Bi

O

and MnCO

). Such a hexaferrite has a dielectric loss lower than

at 9.5 GHz, which is important for microwave applications and possibly for millimeter-wave applications. The paper describes the variation of specific saturation magnetization

and magnetic crystal anisotropy field (

) with temperature (

), and compares the magnetic properties of the sintered hexaferrite with those of the strontium hexaferrite SrFe

O

.