Absolute and relative nonlinear optical coefficients of KDP, KD*P, BaB2O4, LiIO3, MgO:LiNbO3, and KTP measured by phase-matched second-harmonic generation

Both absolute and relative nonlinear optical coefficients of six nonlinear materials measured by second-harmonic generation are discussed. A single-mode, injection-seeded, Q-switched Nd:YAG laser with spatially filtered output was used to generate the 1.064-μm fundamental radiation. The following results were obtained: d₃₆(KD*P)=0.38 pm/V, d₃₆(KD*P)=0.37 pm/V, |d₂₂(BaB ₂O₄)|=2.2 pm/V, d₃₁(LiIO₃ )=-4.1 pm/V, d₃₁(5%MgO:MgO LiNbO₃)=-4.7 pm/V, and d_eff(KTP)=3.2 pm/V. The accuracy of these measurements is estimated to be better than 10%