Oxidation and Removal of NO From Flue Gas by DC Corona Discharge Combined With Alkaline Absorption

Author

Wang, Meiyan ; Zhu, Tianle ; Wang, Hong

Author_Institution

Sch. of Chem. & Environ., Beihang Univ., Beijing, China

Volume

39

Issue

2

fYear

2011

Firstpage

704

Lastpage

710

Abstract

The effects of discharge polarity, discharge electrode configuration, and O₂/CO₂ ratio on NO oxidation by nonthermal plasma (NTP) and NO_x removal by the combination of NTP and alkaline absorption in simulated flue gas were investigated in a combined system of a wire-cylinder plasma reactor and a bubble absorber. The preoxidation of NO by dc corona discharge is effective in promoting the NO_x absorption. Both the NO oxidation efficiency and the NO_x removal efficiency increase with the increase of applied voltage. The positive dc discharge exhibits much higher O₃ formation and NO oxidation performances than the negative one. The increase of the discharge zone length and tooth slice number significantly influences the energy density in the plasma reactor and improves the NO oxidation efficiency for a fixed applied voltage. Increasing the O₂/ CO₂ ratio in the simulated flue gas obviously enhances the NO oxidation and NO_x removal.

Keywords

corona; discharges (electric); flue gases; nitrogen compounds; oxidation; plasma applications; plasma chemistry; DC corona discharge; NO; alkaline absorption; bubble absorber; discharge electrode configuration; discharge polarity; flue gas; nonthermal plasma; oxidation; removal; wire-cylinder plasma reactor; $hbox{NO}_{x}$ removal; Alkaline absorption; NO oxidation; nonthermal plasma (NTP);

fLanguage

English

Journal_Title

Plasma Science, IEEE Transactions on

Publisher

ieee

ISSN

0093-3813

Type

jour

DOI

10.1109/TPS.2010.2092445

Filename

5675693