Title :
Ultrafast dynamics of the heavy fermion state in UX/sub 3/ compounds
Author :
Lobad, A.I. ; Taylor, Antoinette J. ; Sarrao, J.L. ; Trugman, S.A.
Author_Institution :
Div. of Mater. Sci. & Technol., Los Alamos Nat. Lab., NM, USA
Abstract :
Summary form only given. The uranium compounds UX/sub 3/, crystallize in the cubic AuCu/sub 3/-type structure. Due to the wide range of f electron-ligand (X) hybridization strength in these compounds, they exhibit a wide range of behavior: Pauli enhanced paramagnetism (UAl/sub 3/, USi/sub 3/, and UGe/sub 3/), antiferromagnetism (UGa/sub 3/, UPb/sub 3/, and UIn/sub 3/), heavy fermion behavior (USn/sub 3/) and superconductivity (URu/sub 3/). The interaction of the partially filled f shell electrons with the conduction electrons causes the mass renormalization of the latter and the formation of heavy quasiparticles. We investigate the dynamics of this renormalization in UX/sub 3/ compounds, where X=Al, Ga, Sn with electronic specific heat coefficients (/spl gamma/) of 43 mJ/molK/sup 2/, 52 mJ/molK/sup 2/, and 172 mJ/molK/sup 2/ respectively, (as compared to /spl gamma//spl sim/1 mJ/molK/sup 2/ for ordinary metals such as Cu). The single crystals of UX/sub 3/ were grown using a standard flux technique.
Keywords :
aluminium alloys; gallium alloys; heavy fermion systems; high-speed optical techniques; reflectivity; renormalisation; specific heat; tin alloys; uranium alloys; Pauli enhanced paramagnetism; UAl/sub 3/; UGa/sub 3/; UGe; UGe/sub 3/; UIn/sub 3/; UPb/sub 3/; URu/sub 3/; USi/sub 3/; USn/sub 3/; UX/sub 3/ compounds; antiferromagnetism; conduction electrons; cubic AuCu/sub 3/-type structure; electronic specific heat coefficients; f electron-ligand hybridization strength; heavy fermion behavior; heavy fermion state; heavy quasiparticles; mass renormalization; partially filled f shell electrons; renormalization; single crystals; standard flux technique; superconductivity; ultrafast dynamics; Delay; Electrons; Magnetic materials; Magnetization; Optical films; Optical pumping; Polarimetry; Signal resolution; Ultrafast electronics; Ultrafast optics;
Conference_Titel :
Quantum Electronics and Laser Science Conference, 2000. (QELS 2000). Technical Digest
Conference_Location :
San Francisco, CA, USA
Print_ISBN :
1-55752-608-7