Title :
Production of Ammonia by Heterogeneous Catalysis in a Packed-Bed Dielectric-Barrier Discharge: Influence of Argon Addition and Voltage
Author :
Jungmi Hong ; Prawer, S. ; Murphy, Anthony B.
Author_Institution :
Mater. Sci. & Eng., CSIRO, Lindfield, NSW, Australia
Abstract :
Ammonia was synthesized from nitrogen and hydrogen in a dielectric-barrier discharge reactor packed with glass spheres and MgO pellets at atmospheric pressure. The addition of argon to nitrogen and hydrogen, and increasing the peak voltage, led to increases in discharge power and uniformity, gas temperature, and the fraction of hydrogen converted to ammonia.
Keywords :
ammonia; argon; catalysis; dielectric-barrier discharges; hydrogen; nitrogen; plasma applications; Ar; H2; MgO pellets; NH2; O2; ammonia production; argon; heterogeneous catalysis; hydrogen; nitrogen; packed-bed dielectric-barrier discharge reactor; Argon; Dielectrics; Discharges (electric); Plasma temperature; Production; Temperature measurement; Heterogeneous ammonia production; packed-bed dielectric barrier discharge; plasma catalysis; plasma catalysis.;
Journal_Title :
Plasma Science, IEEE Transactions on
DOI :
10.1109/TPS.2014.2323077