An Experiment Using High Spectral Resolution CrIS Measurements for Atmospheric Trace Gases: Carbon Monoxide Retrieval Impact Study

We perform a demonstration experiment using the National Oceanic Atmospheric Administration Unique Cross-track Infrared Sounder (CrIS)/Advanced Technology Microwave Sounder Processing System to assess the improvement on trace gas retrievals upon switching to high spectral resolution CrIS radiance measurements (0.625 cm^-1). The focus of this study is carbon monoxide retrievals. The experimental high spectral resolution CO retrievals show a remarkable improvement, of almost up to one order of magnitude in the degree of freedom of the signal, with respect to the low-resolution mode. Furthermore, high-resolution CO retrievals show similar skill with respect to existing CO operational products from the Atmospheric InfraRed Sounder, Atmospheric Sounder Interferometer, and Measurements of Pollution In The Troposphere instruments, both in terms of spatial variability and degrees of freedom. The results of this research provide evidence to support the need for high spectral resolution CrIS measurements. This is a fundamental prerequisite in guaranteeing continuity to the CO afternoon orbit monitoring as part of a multisatellite uniformly integrated long-term data record of atmospheric trace gases.