• DocumentCode
    1806770
  • Title

    Computer Simulation of the Anisotropy of Fluorescence in Ring Molecular Systems: Influence of Disorder and Ellipticity

  • Author

    Herman, Pavel ; Zapletal, David ; Barvik, Ivan

  • Author_Institution
    Dept. of Phys., Univ. of Hradec Kralove, Hradec Kralove, Czech Republic
  • Volume
    1
  • fYear
    2009
  • fDate
    29-31 Aug. 2009
  • Firstpage
    437
  • Lastpage
    442
  • Abstract
    We use massively parallelized system for computer simulation of time dependence of the anisotropy of fluorescence for the ring LH2 from Rhodopseudomonas acidophila with tangential optical transition dipole arrangements. Different models of uncorrelated static disorder and also ellipticity (correlated static disorder) in local molecular energies are taken into account. Dynamical disorder, interaction with a bath, is included in Markovian approximation of the equations of motion for the so called exciton density matrix. In this paper we compare the results for two different models of the spectral density of phonon bath.
  • Keywords
    Markov processes; approximation theory; bioinformatics; molecular biophysics; Markovian approximation; computer simulation; exciton density matrix; massively parallelized system; phonon bath; rhodopseudomonas acidophila; ring molecular systems; tangential optical transition dipole arrangements; uncorrected static disorder; Anisotropic magnetoresistance; Computer simulation; Equations; Excitons; Fluorescence; Geometrical optics; Mathematics; Microorganisms; Physics; Ultrafast optics; LH2 ring; anisotropy of fluorescence; coherence; exciton;
  • fLanguage
    English
  • Publisher
    ieee
  • Conference_Titel
    Computational Science and Engineering, 2009. CSE '09. International Conference on
  • Conference_Location
    Vancouver, BC
  • Print_ISBN
    978-1-4244-5334-4
  • Electronic_ISBN
    978-0-7695-3823-5
  • Type

    conf

  • DOI
    10.1109/CSE.2009.88
  • Filename
    5283389