Temporal off-diagonal long-range order in polariton condensates

Summary form only given. Bosons can populate quantum states macroscopically, forming various kinds of thermal-equilibrium, and quasi-equilibrium condensates, which exhibit a wide range of collective phenomena including superfluidity and macroscopic coherence in matter. Interferometry has been employed to demonstrate long-range off-diagonal order in cold-atom systems, and, recently, in the rapidly developing field of exciton-polariton condensates. However, all such interferometric measurements have been performed on steady-state condensates, unable to access the temporal off-diagonal order and non-equilibrium dynamics. Moreover, in solid-state systems, interference between two separate condensates has not been observed before. Here we use optical injection to resonantly generate two dynamic exciton-polariton condensates with distinct momenta and at different times. We characterize the interference between condensates, demonstrating their long-range temporal order. We show that the build-up of the temporal long-range order strongly depends on the strength of polariton interactions, as well as the temperature and particle density. Moreover, polariton interactions yield a blue shift of the dynamic condensate energy, acting as an extremely large optical nonlinearity. These results provide direct evidence of temporal long-range order in dynamic condensates as well as demonstrate a new approach for probing the ultrafast coherent dynamics of exciton-polaritons, opening new directions in the fundamental study of coherence in matter as well as in practical applications such as quantum information processing and ultrafast logic.