Title :
Generation of Reactive Oxygen Species in Helium–Oxygen Radio-Frequency Discharges at Atmospheric Pressure
Author :
Jin He ; Yuantao Zhang
Author_Institution :
Shandong Provincial Key Lab. of UHV Technol. & Gas Discharge Phys., Shandong Univ., Jinan, China
Abstract :
Reactive oxygen species (ROS) generated in atmospheric plasmas are believed to play an important role in plasma medicine and related areas. In this paper, we explored a fluid model to investigate the production and destruction of ROS in atmospheric radio-frequency (RF) discharges with helium-oxygen mixture as working gas; to speed up the computation, only 17 species and 48 reactions are considered in plasmas. At a given applied voltage, the variations of ROS depending on the oxygen admixture are discussed and the key reactions related to the generation of ROS are further confirmed. Through increasing the applied voltage, the evolution of ROS based on the simulation results are also given. The simulation data agree well with the experimental measurements.
Keywords :
gas mixtures; helium; high-frequency discharges; oxygen; plasma applications; plasma chemistry; plasma simulation; He-O2; applied voltage; helium-oxygen radio-frequency discharges; oxygen admixture; plasma medicine; pressure 1 atm; reactive oxygen species; Atmospheric modeling; Computational modeling; Current density; Discharges (electric); Helium; Plasmas; Radio frequency; Atmospheric radio-frequency (RF) discharges; plasma chemistry; plasma simulation; reactive oxygen species (ROS);
Journal_Title :
Plasma Science, IEEE Transactions on
DOI :
10.1109/TPS.2013.2279678