Title :
Strong mid-infrared transient absorption of one-dimensional copper oxide Sr/sub 2/CuO/sub 3/
Author :
Ashida, M. ; Uchida, S. ; Tokura, Y. ; Kuwata-Gonokami, M.
Author_Institution :
Exploratory Res. for Adv. Technol., Japan Sci. & Technol. Corp., Kawasaki, Japan
Abstract :
Summary form only given. Electron correlation effects, which have attracted much interest after the discovery of high temperature superconductivity and manifest themselves in anomalous transport and/or magnetic phenomena, can also be found in optical properties of strongly correlated electron systems. In particular, we have recently discovered strong optical nonlinearity of one-dimensional Mott insulator Sr/sub 2/CuO/sub 3/ in near-infrared (IR) region. Importantly, the material shows picosecond recovery of the optical transparency making it possible to employ this material in ultrafast all-optical switching devices. However, the relaxation dynamics of the optical excited states is still unclear. To investigate the relaxation process, we performed pump-probe transmission measurements in mid- and near-IR region of 0.1-1 eV. We have found anomalously strong transient absorption band at 0.3 eV.
Keywords :
absorption coefficients; infrared spectra; strongly correlated electron systems; strontium compounds; time resolved spectra; two-photon spectra; Sr/sub 2/CuO/sub 3/; absorption coefficient; instantaneous pump-induced absorption change; one-dimensional Mott insulator; one-photon absorption spectra; optical excited states; optical transparency; picosecond recovery; pump-probe transmission measurements; relaxation process; spin degree of freedom; spin excited states; spinon sideband; strong mid-infrared transient absorption; strong optical nonlinearity; strongly correlated electron systems; two-photon absorption spectra; Infrared spectroscopy;
Conference_Titel :
Quantum Electronics and Laser Science Conference, 2002. QELS '02. Technical Digest. Summaries of Papers Presented at the
Conference_Location :
Long Beach, CA, USA
Print_ISBN :
1-55752-708-3
DOI :
10.1109/QELS.2002.1031305