• DocumentCode
    2536635
  • Title

    Construction of an ESR-STM for single molecular based magnets anchored at surfaces

  • Author

    Messina, Paolo ; Sigalotti, Paolo ; Lenci, Lorenzo ; Prato, Stefano ; Gatteschi, Dante

  • Author_Institution
    INSTM Unita´´ di Firenze, Sesto Fiorentino, Italy
  • fYear
    2004
  • fDate
    16-19 Aug. 2004
  • Firstpage
    642
  • Lastpage
    644
  • Abstract
    Reading and manipulating the spin status of single magnetic molecules is of paramount importance both for applicative and fundamental purposes. The possibility to combine electron spin resonance (ESR) and scanning tunnelling microscopy (STM) has been explored one decade ago. A few experiments have raised the question whether or not an EPR spectrum of single molecule is detachable. Only a few data have been reported in modern surface science literature. To date it has yet to be proven till which extent ESR can be reliably and reproducibly performed on single molecules. We are setting up a new ESR-STM "spectrometer" to verify and study the effect of spin-spin correlations in the frequency spectrum of the tunneling current which flows through a single magnetic adsorbate and a metal surface. Here, we discuss, the major experimental challenges that we are attempting to overcome.
  • Keywords
    EPR spectrometers; magnetic tunnelling; molecular magnetism; scanning tunnelling microscopy; spin-spin interactions; EPR spectrum; ESR-STM spectrometer; electron spin resonance; frequency spectrum; metal surface; scanning tunnelling microscopy; single magnetic adsorbates; single molecular based magnets; spin status; spin-spin correlations; tunneling current; Instruments; Magnetic field measurement; Magnetic fields; Magnetic resonance; Magnets; Molecular electronics; Paramagnetic resonance; Radio frequency; Signal design; Tunneling;
  • fLanguage
    English
  • Publisher
    ieee
  • Conference_Titel
    Nanotechnology, 2004. 4th IEEE Conference on
  • Print_ISBN
    0-7803-8536-5
  • Type

    conf

  • DOI
    10.1109/NANO.2004.1392446
  • Filename
    1392446