DocumentCode
2655552
Title
Femtosecond hydrogen bond dynamics by spectrally- and time-resolved vibrational sum frequency generation
Author
Bordenyuk, Andrey N. ; Benderskii, Alexander V.
Author_Institution
Dept. of Chem., Wayne State Univ., Detroit, MI, USA
Volume
3
fYear
2005
fDate
22-27 May 2005
Firstpage
1884
Abstract
Time- and frequency-domain 3-wave mixing spectroscopy is developed as a surface-selective nonlinear technique capable of measuring spectral evolution of vibrational coherences. Hydrogen bond dynamics of interfacial water is observed to proceed on 100 fs timescale.
Keywords
high-speed optical techniques; hydrogen bonds; multiwave mixing; optical frequency conversion; vibrational states; 100 fs; 3-wave mixing; femtosecond hydrogen bond dynamics; frequency-domain spectroscopy; interfacial water; spectral evolution; surface-selective nonlinear technique; time-resolved vibrational sum frequency generation; vibrational coherences; Bonding; Delay effects; Frequency measurement; Hydrogen; Optical pulses; Optical surface waves; Polarization; Spectroscopy; Ultrafast optics; Vibration measurement;
fLanguage
English
Publisher
ieee
Conference_Titel
Quantum Electronics and Laser Science Conference, 2005. QELS '05
Print_ISBN
1-55752-796-2
Type
conf
DOI
10.1109/QELS.2005.1549316
Filename
1549316
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