Molecular Spectroscopy With a Compact 557-GHz Heterodyne Receiver

We report on a heterodyne terahertz spectrometer based on a fully integrated 557-GHz receiver and a digital fast Fourier transform spectrometer. The receiver consists of a chain of multipliers and power amplifiers, followed by a heterostructure barrier varactor tripler that subharmonically pumps a membrane GaAs Schottky diode mixer. All sub-components are newly developed and optimized with regard to the overall receiver performance such as noise temperature, power consumption, weight and physical size. The receiver works at room temperature, has a double sideband noise temperature as low as 2000 K at a maximum power consumption of 4.5 W with an Allan time of 10 s and a sideband gain ratio of 0.52. The performance of the spectrometer is demonstrated by absorption spectroscopy of H₂O and CH₃OH with an instantaneous bandwidth of 1.5 GHz and a resolution of 183 kHz. Several pressure broadening parameters of methanol absorption lines were determined, that agree with other published data. Using the experimentally determined molecular parameters the CH₃OH absorption spectrum could be modeled with very high precision.