Title :
Optimizing Flux Pinning of
(YBCO) Thin Films With Unique Large Nanoparticle Size and High Concentration of <
Author :
Sebastian, Mary Ann P. ; Reichart, Joshua N. ; Ratcliff, Margaret M. ; Burke, Jack L. ; Haugan, Timothy J. ; Chen-Fong Tsai ; Haiyan Wang
Author_Institution :
Air Force Res. Lab., Wright Patterson Air Force Base (AFB), Dayton, OH, USA
Abstract :
Addition of second-phase nanosize defects to YBa2Cu3O7-δ (YBCO) superconductor thin films is known to enhance flux pinning and increase current densities (Jc). The addition of Y2BaCuO5 (Y211) was previously studied in (Y211/ YBCO)N multilayer structures and in Y211 + YBCO films deposited from pie-shaped targets. This research systematically studies the effect of Y211 addition in thin films deposited by pulsed laser deposition from YBCO1-xY211x(x = 0-15 vol.%) single targets, at temperatures of 785°C-840°C. Interestingly, the resulting size of Y211 particles is 20-40 nm, in contrast to 10-15 nm in previous studies of Y211 and 5-10 nm for other second-phase defect additions, and the number density is reduced. A slight increase of Jc(H, T) was achieved, compared with previous optimization studies. Results and comparisons of flux pinning, intrinsic stresses imaged by TEM, current densities, critical temperatures, and microstructures will be presented. The overall low intrinsic stress on YBCO from Y211 lattice mismatch is smaller than previously studied second-phase defect additions known, which is hypothesized to be the driving force in achieving the unusually large second-phase nanoparticle size and volume fraction thus far in YBCO thin films.
Keywords :
barium compounds; critical current density (superconductivity); crystal microstructure; flux pinning; high-temperature superconductors; nanoparticles; particle size; pulsed laser deposition; superconducting thin films; superconducting transition temperature; transmission electron microscopy; yttrium compounds; TEM; Y211 additions; YBCO-Y2BaCuO5; critical temperatures; current densities; flux pinning; intrinsic stresses; lattice mismatch; microstructures; multilayer structures; number density; pulsed laser deposition; second-phase nanoparticle size; second-phase nanosize defects; superconductor thin films; temperature 785 degC to 840 degC; Current density; Films; Flux pinning; Lattices; Nanoparticles; Yttrium barium copper oxide; Critical current density; Flux pinning; High-temperature superconductors; Yttrium barium copper oxide; flux pinning; high-temperature superconductors; yttrium barium copper oxide;
Journal_Title :
Applied Superconductivity, IEEE Transactions on
DOI :
10.1109/TASC.2014.2368072