Title :
Cavity-enhanced sideband cooling of molecules to the ground state of a harmonic trap
Author :
Kowalewski, Markus ; Morigi, Giovanna ; Pinkse, Pepijn W H ; De Vivie-Riedle, Regina
Author_Institution :
Dept. fur Chem. und Biochem., Ludwig-Maximilians-Univ. Munchen, Munich, Germany
Abstract :
A new approach for cavity-mediated optical cooling of molecules in harmonic traps is investigated using vibrational transitions in the infrared regime. Ab initio methods are used to determine transition dipole moments of the rovibrational modes, the lifetime of the rovibrational states and the polarizabilities. Theoretical results predict cooling of molecular ions into the ground state of the trap on a sub-milisecond time scale.
Keywords :
ab initio calculations; ground states; laser cooling; molecular moments; polarisability; rotational-vibrational states; vibrational states; ab initio method; cavity-enhanced sideband cooling; cavity-mediated optical cooling; ground state; harmonic trap; infrared regime; molecular ions; polarizabilities; rovibrational modes; rovibrational states; submilisecond time scale; transition dipole moments; vibrational transitions; Astrochemistry; Atomic beams; Charge carrier processes; Chemical lasers; Cooling; Laser theory; Laser transitions; Optical resonators; Particle beam optics; Stationary state;
Conference_Titel :
Lasers and Electro-Optics 2009 and the European Quantum Electronics Conference. CLEO Europe - EQEC 2009. European Conference on
Conference_Location :
Munich
Print_ISBN :
978-1-4244-4079-5
Electronic_ISBN :
978-1-4244-4080-1
DOI :
10.1109/CLEOE-EQEC.2009.5192359