Title :
Observation of intra-molecular vibrational dynamics using high-harmonic generation as a probe
Author :
Wagner, Nick ; Wüest, Andrea ; Kapteyn, Henry ; Murnane, Margaret
Author_Institution :
JILA, Univ. of Colorado, Boulder, CO
Abstract :
As one of the first observations of intra-molecular dynamics using high-order harmonic generation, we impulsively excite vibrations in SF6 and observe oscillations in the intensity of high-order harmonic emission from these molecules.
Keywords :
intramolecular mechanics; optical harmonic generation; oscillations; probes; sulphur compounds; SF6; high-order harmonic generation; intramolecular vibrational dynamics; oscillations; probe; vibration excitation; Data mining; Delay effects; Optical harmonic generation; Probes; Pulse modulation; Spectroscopy; Stimulated emission; Sulfur hexafluoride; Ultrafast optics; Ultraviolet sources; (320.7120) Ultrafast phenomena; (320.7150) Ultrafast spectroscopy;
Conference_Titel :
Lasers and Electro-Optics, 2006 and 2006 Quantum Electronics and Laser Science Conference. CLEO/QELS 2006. Conference on
Conference_Location :
Long Beach, CA
Print_ISBN :
978-1-55752-813-1
Electronic_ISBN :
978-1-55752-813-1
DOI :
10.1109/CLEO.2006.4628439
