Title : 
Critical slowing down and off-resonant enhancement of avalanche nonlinearities
         
        
            Author : 
Shu, Q. ; Rand, S.C.
         
        
            Author_Institution : 
Div. of Appl. Phys., Michigan Univ., Ann Arbor, MI, USA
         
        
        
        
        
        
            Abstract : 
We report two-beam coupling measurements of temporal response and intensity-dependent index changes in the avalanche crystal LiYF/sub 4/:Tm(3+). Surprisingly, the induced nonlinear response on the excited state resonance is dominated by a real portion arising from a non-resonant ground state transition. Critical slowing down of excited state dynamics is also predicted and observed.
         
        
            Keywords : 
excited states; lithium compounds; multiwave mixing; optical materials; refractive index; thulium; LiYF/sub 4/:Tm; LiYF/sub 4/:Tm(3+); avalanche crystal; avalanche nonlinearities; excited state dynamics; excited state resonance; induced nonlinear response; intensity-dependent index changes; non-resonant ground state transition; off-resonant enhancement; temporal response; two-beam coupling measurements; Delay effects; Laser excitation; Multilevel systems; Nonlinear optics; Physics; Probes; Refractive index; Resonance; Stationary state; Wavelength measurement;
         
        
        
        
            Conference_Titel : 
Quantum Electronics and Laser Science Conference, 1996. QELS '96., Summaries of Papers Presented at the
         
        
            Conference_Location : 
Anaheim, CA, USA
         
        
            Print_ISBN : 
1-55752-444-0