Title :
Dissociative ionization dynamics of ethanol as studied by chirped intense laser pulses
Author :
Itakura, R. ; Yamanouchi, K. ; Tanabe, T. ; Okamoto, T. ; Kannari, F.
Author_Institution :
Dept. of Chem., Tokyo Univ., Japan
Abstract :
Dynamics of the dissociative ionization of ethanol in an intense laser field has been studied by changing the linear chirp rate of the intense laser pulse. The relative yields of fragment ions exhibit strong dependences on the chirp rate. Since the direction of the chirp does not influence the relative yields, the temporal pulse duration is considered to be a key factor for determining the branching of the reaction pathways.
Keywords :
chirp modulation; high-speed optical techniques; molecule-photon collisions; organic compounds; photodissociation; photoionisation; chirped intense laser pulses; dissociative ionization; ethanol; fragment ions; linear chirp rate; relative yields; temporal pulse duration; Chemical lasers; Chirp; Ethanol; Ionization; Laser theory; Laser transitions; Optical design; Optical pulse shaping; Optical pulses; Pulse amplifiers;
Conference_Titel :
Lasers and Electro-Optics, 2003. CLEO/Pacific Rim 2003. The 5th Pacific Rim Conference on
Print_ISBN :
0-7803-7766-4
DOI :
10.1109/CLEOPR.2003.1277286