Title :
High-Purity CdMnTe Radiation Detectors: A High-Resolution Spectroscopic Evaluation
Author :
Rafiei, Ramin ; Reinhard, Mark I. ; Kim, Kunsu ; Prokopovich, Dale A. ; Boardman, D. ; Sarbutt, A. ; Watt, G.C. ; Bolotnikov, A.E. ; Bignell, Lindsey J. ; James, Ralph B.
Author_Institution :
Australian Nucl. Sci. & Technol. Organ., Sydney, NSW, Australia
Abstract :
The charge transport properties of a high-purity CdMnTe (CMT) crystal have been measured at room temperature down to a micron-scale resolution. The CMT crystal, doped with indium, was grown by the vertical Bridgman technique. To reduce the residual impurities in the Mn source material, the growth process incorporated a five-times purification process of MnTe by a zone-refining method with molten Te solvent. The resulting 2.6 mm thick crystal exhibited an electron mobility-lifetime product of μnτn=2.9 × 10-3 cm2V-1. The velocity of electron drift was calculated from the rise time distribution of the preamplifier´s output pulses at each measured bias. The electron mobility was extracted from the electric field dependence of the drift velocity and at room temperature it has a value of μn=(950±90) cm2/Vs. High-resolution maps of the charge collection efficiency have been measured using a scanning microbeam of 5.5 MeV 4He2+ ions focused to a beam diameter <; 1 μm and display large-area spatial uniformity. The evolution of charge collection uniformity across the detector has been highlighted by acquiring measurements at applied biases ranging between 50 V and 1100 V. Charge transport inhomogeneity has been associated with the presence of bulk defects. It has been demonstrated that minimizing the content of impurities in the MnTe source material is highly effective in achieving major improvements in the CMT detector´s performance as compared to previous data.
Keywords :
II-VI semiconductors; cadmium compounds; carrier lifetime; crystal growth from melt; crystal purification; electron mobility; manganese compounds; preamplifiers; semiconductor counters; semiconductor growth; zone refining; He2+ ions; Mn source material; beam diameter; bulk defects; charge collection efficiency; charge transport inhomogeneity; electron drift velocity; electron mobility-lifetime product; high-purity CdMnTe radiation detectors; high-resolution spectroscopic evaluation; large-area spatial uniformity; molten Te solvent; preamplifier output pulses; residual impurities; rise time distribution; size 2.6 mm; temperature 293 K to 298 K; vertical Bridgman technique; zone-refining method; Crystals; Detectors; Electrodes; Electron mobility; Pulse measurements; Semiconductor device measurement; Temperature measurement; CMT; Carrier lifetime; CdMnTe; IBIC; charge collection efficiency; compound semiconductor radiation detector; crystal growth; drift velocity; manganese purity; mobility; mobility-lifetime;
Journal_Title :
Nuclear Science, IEEE Transactions on
DOI :
10.1109/TNS.2013.2243167