• DocumentCode
    69680
  • Title

    Hydrogen Production From Partial Oxidation of Methane Using an AC Rotating Gliding Arc Reactor

  • Author

    Xiao Dong Li ; Hao Zhang ; Shi Xin Yan ; Jian Hua Yan ; Chang Ming Du

  • Author_Institution
    Inst. for Thermal Power Eng., Zhejiang Univ., Hangzhou, China
  • Volume
    41
  • Issue
    1
  • fYear
    2013
  • fDate
    Jan. 2013
  • Firstpage
    126
  • Lastpage
    132
  • Abstract
    Hydrogen, as well as petrochemical feedstock, can be produced by the partial oxidation of methane in an alternating-current rotating-gliding-arc plasma driven by swirling flow. The effects of the air ratio (0.6 to 1.6), height of outer cover (25 and 45 cm), supply voltage (6.6 to 11.1 kV), and gas flow rate (6 to 18 L/min) on methane reforming have been investigated. The conversion of methane grows with rising air ratio, whereas hydrogen selectivity first augments and then declines. A higher outer cover was beneficial, and maximum methane conversion attains 80.73%. Higher voltage improves the reactor performance. As gas flow rate grows, both methane conversion and hydrogen selectivity diminish, while power consumption first drops to a minimum value of 8.23 kJ/L H2 for a flow rate of 16 L/min and then again amplifies.
  • Keywords
    arcs (electric); chemical reactors; hydrogen production; organic compounds; oxidation; plasma applications; plasma chemistry; plasma sources; AC rotating gliding arc reactor; H2; air ratio effects; alternating current rotating gliding arc plasma; altitude 25 cm; altitude 45 cm; gas flow rate effects; hydrogen production; hydrogen selectivity; methane conversion; methane partial oxidation; methane reforming; outer cover height effects; petrochemical feedstock; supply voltage effects; swirling flow; voltage 6.6 kV to 11.1 kV; Electrodes; Hydrogen; Inductors; Oxidation; Plasmas; Power demand; Production; Hydrogen; methane; partial oxidation; plasma; rotating gliding arc (RGA);
  • fLanguage
    English
  • Journal_Title
    Plasma Science, IEEE Transactions on
  • Publisher
    ieee
  • ISSN
    0093-3813
  • Type

    jour

  • DOI
    10.1109/TPS.2012.2226608
  • Filename
    6353986