Title :
Thermoluminescence of Cs2 LiYCl6, Cs2LiYCl 6:Ce3+ and Cs2LiYCl6:Pr 3+ Crystals
Author :
Van Loef, Edgar V. ; Higgins, William M. ; Squillante, Michael R. ; Shah, Kanai S.
Author_Institution :
Radiat. Monitoring Devices, Watertown
fDate :
6/1/2007 12:00:00 AM
Abstract :
In this paper we report on the thermoluminescence of Cs2LiYCI6, Cs2LiYCl6:Ce3+ and Cs2LiYCl6:Pr3+ crystals. Low-temperature glow curves and isothermal decay spectra are presented. All three crystals exhibit prominent glow peaks below 300 K. The Cs2LiYCl6 sample shows a major peak at 58 K in addition to a broad band between 75 K and 150 K. The glow curve of Cs2LiYCl6:Pr3+ is similar to that of Cs2LiYCl6 but shows additional peaks at 222 K and 277 K. The glow curve of Cs2LiYCl6:Ce3+ is dominated by a major glow peak at 214 K with minor peaks at 50 K and 88 K. Lifetimes of traps derived from isothermal decay spectra measured at the temperature maximum of selected glow peaks are of the order of tens of seconds.
Keywords :
caesium compounds; cerium; lithium compounds; praseodymium; solid scintillation detectors; thermoluminescence; yttrium compounds; Cs2LiYCI6 - System; Cs2LiYCI6 crystal; Cs2LiYCl6:Ce - System; Cs2LiYCl6:Ce3+ crystal; Cs2LiYCl6:Pr - System; Cs2LiYCl6:Pr3+ crystal; glow curves; isothermal decay spectra; temperature 214 K; temperature 222 K; temperature 277 K; temperature 50 K; temperature 58 K; temperature 75 K to 150 K; temperature 88 K; thermoluminescence; trap lifetime; Crystalline materials; Crystallization; Crystals; Electron traps; Heating; Isothermal processes; Luminescence; Neutrons; Temperature measurement; Time measurement; Cs$_{2}$LiYCl$_{6}$; elpasolites; scintillation detectors; thermoluminescence;
Journal_Title :
Nuclear Science, IEEE Transactions on
DOI :
10.1109/TNS.2007.896216