Climatology of the Aerosol Extinction-to-Backscatter Ratio from Sun-Photometric Measurements

The elastic lidar equation contains two unknown atmospheric parameters, namely, the particulate optical extinction and backscatter coefficients, which are related through the lidar ratio (i.e., the particulate-extinction-to-backscatter ratio). So far, independent inversion of the lidar signal has been carried out by means of Raman lidars (usually limited to nighttime measurements), high-spectral-resolution lidars, or scanning elastic lidars under the assumption of a homogeneously vertically stratified atmosphere. In this paper, we present a procedure to obtain the lidar ratio at 532 nm by a combined Sun-photometer-aerosol-model inversion, where the viability of the solution is largely reinforced by assimilating categorized air-mass back-trajectory information. Thus, iterative lidar-ratio tuning to reconstruct the Sun-photometric aerosol optical depth (AOD) is additionally constrained by the air-mass back trajectories provided by the hybrid single-particle Lagrangian integrated-trajectory model. The retrieved lidar ratios are validated with inversions of lidar data based on the Klett-Fernald-Sasano algorithm and with the Aerosol Robotic Network (AERONET)-retrieved lidar ratios. The estimated lidar ratios concur with the AERONET-retrieved lidar ratios and with those of the well-known KFS inversion constrained with Sun-photometric AOD values and embedded single-scattering models. The proposed method can be applied to routinely extract climatological values of the lidar ratio using measurements of direct solar irradiance (more numerous than those of sky radiance).