Title :
Quantum coherence controls the charge separation in a prototypical artificial light harvesting system
Author :
Falke, S.M. ; Rozzi, C.A. ; Spallanzani, N. ; Rubio, A. ; Molinari, E. ; Brida, D. ; Maiuri, M. ; Cerullo, G. ; Schramm, H. ; Christoffers, J. ; Lienau, C.
Author_Institution :
Carl von Ossietzky Univ. Oldenburg, Oldenburg, Germany
Abstract :
Ultrafast spectroscopy and quantum-dynamics simulations of an artificial supramolecular light-harvesting system give strong evidence that the quantum-correlated wavelike motion of electrons and nuclei governs the ultrafast electronic charge transfer.
Keywords :
charge exchange; energy harvesting; high-speed optical techniques; optical control; organic compounds; quantum optics; spectroscopy; artificial supramolecular light-harvesting system; charge separation; prototypical artificial light harvesting system; quantum coherence controls; quantum-correlated wavelike motion; quantum-dynamics simulations; ultrafast electronic charge transfer; ultrafast spectroscopy; Charge transfer; Dynamics; Nonlinear optics; Oscillators; Spectroscopy; Ultrafast electronics; Ultrafast optics;
Conference_Titel :
Lasers and Electro-Optics (CLEO), 2012 Conference on
Conference_Location :
San Jose, CA
Print_ISBN :
978-1-4673-1839-6
